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High Temperature Electrical Properties of Barium Zirconate-Cerate Type Proton-Conducting Ceramics

Thursday, 2 June 2016: 08:40
Indigo Ballroom C (Hilton San Diego Bayfront)
H. Shimada, T. Yamaguchi, H. Sumi, and Y. Fujishiro (National Institute of AIST)
We have investigated electrochemical ceramic cells such as fuel cells and electrolysis cells using perovskite-type proton-conducting ceramics for electrolyte material. In particular, we focus on Barium zirconate-cerate (Ba(ZrCe)O3) type proton-conducting ceramics, which have high protonic conductivity and chemical stability. Many researchers have used these materials for proton-conducting solid oxide fuel cells (SOFCs) and have reported good performance. We have also obtained similar good performance in electrochemical measurements using anode-supported SOFCs. However, the bulk conductivity of Ba(ZrCe)O3 showed a significant change around 700°C. In this study, we discussed the change in the conductivity related to the transport number and the thermal expansion behaviors.