1685
The Electrochemical Behaviour of Some Composite Coatings Obtained By Electrodeposition on Metallic Substrate

Wednesday, 1 June 2016
Exhibit Hall H (San Diego Convention Center)

ABSTRACT WITHDRAWN

Nanocomposite films based on 3,4 ethylen-dioxythiophene and 3-methylthiophene with functionalized single-walled carbon nanotubes (SWANTs- polyaminobenzene sulfonic acid - CNT-PABS, SWANTs- with carboxylic acids functionalized - CNT-COOH) and different large anionic surfactants as dopants (1-dodecane sulfonic acid sodium salt, sodium dioctyl sulfosuccinate - AOT and sodium dodecylbenzenesulfonate - SDBS) were studied. It was fabricated by a simple oxidative electropolimerization method.

All the obtained composites showed improved mechanical integrity, higher electronic and ionic conductivity and exhibited larger electrode specific capacitance than the polymer alone. These nanoporous composite films were grown electrochemically from aqueous solutions such that constituents were deposited simultaneously onto substrate electrode.

The synthetic, morphological and electrical properties of the obtained nanocomposite films were compared. Scanning electron microscopy (SEM) revealed that the composite films consisted of nanoporous networks of SWCNTS (single-walled carbon nanotubes) coated with polymeric film. Cyclic voltammetry (CV) and electrochemical impedance spectroscopy (EIS) demonstrated that these composite films had similar electrochemical response rates to pure polymeric films but a lower resistance and much improved mechanical integrity. The large anionic surfactants served as dopant during the electropolymerization to synthesize polymer/CNTSF composite films. The electrochemical and physical properties of the resulting composites were evaluated by cyclic voltammetry (CV), electrochemical impedance spectroscopy (EIS) and FT-IR spectroscopy techniques. The improved properties of the electrodes were obtained by using these composite films. The specific electrochemical capacitance of the composite films is a significantly greater value than that for pure polymer films prepared similarly. All of the composite films were a very promising electrode material for application in supercapacitor.